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The project aims at producing an ENVISAT-1 mission-long monitoring of the inorganic chlorine (Cly) and fluorine (Fy) loading in the Earth’s middle atmosphere, based on FTIR vertical column abundance measurements of the key related species HCl, ClONO2, HF and COF2 at 10 ground-based NDSC sites distributed worldwide. These Cly and Fy inventories will be completed with ClO and OClO measurements expected as Level-2 products from ENVISAT-1. The column abundances of the source gases CFC-12 and HCFC-22 will be used to place the stratospheric Cly and Fy evolution in perspective with the more complete sets of organic chlorinated and fluorinated compounds measured at the ground by the in situ networks NOAA-CMDL and AGAGE. The assimilation of the retrieved geophysical data bases will be performed through 3-D model calculations incorporating physical, chemical and transport characteristics of the global atmosphere.
The present project aims at the geophysical validation, from pole to pole and on the long term, of key ozone-related level-2 products (O3, NO2, BrO, OClO, and ClO) from GOMOS, MIPAS and SCIAMACHY onboard ENVISAT-1, and at a contribution to the maturation of the related level-1b-to-2 data processors. Application data processing will be used to convert level-2 data into a more suitable format for validation and scientific end-users. The respective performances of the ENVISAT data products, and their sensitivity to various relevant parameters, will be investigated from the Arctic to the Antarctic, over a variety of geophysical conditions. The impact of these performances on specific atmospheric chemistry studies will be emphasised. The pseudo-global investigations will rely on correlative studies of ENVISAT data with high-quality ground-based, in situ and balloon observations associated with the Network for the Detection of Stratospheric Change (NDSC).
The project will provide a long-term, pseudo-global validation support to the ENVISAT-1 atmospheric measurements, based on mutually consistent high-quality solar and lunar observations from FTIR spectrometers operated at primary and a number of complementary NDSC stations. The validation is limited to a number of target species, most of which are primary NRT or OL level-2 products of the mission, with focus on NOy components: O3, NO2, NO, N2O, HNO3, HNO4, H2CO, CO and CH4. Synergistic use will be made of column and profile data from MIPAS, GOMOS and SCIAMACHY. The ground network will deliver mean vertical column abundances for all target species with NDSC-type quality, and height profile information for some target gases as secondary products to the PI's home institute, where the correlative analyses with the ENVISAT-1 products will be done. Asynoptic mapping tools will support the validation efforts.