Projects/Activities

The submitted proposal aims to perform the monitoring of the pollen rain in the Greenland atmosphere by distinguishing the local pollen production, relatively low, from pollen grains originating from other Arctic areas. A regular monitoring of the atmospheric pollen content must be performed in order to evaluate the amount emitted and characterise the seasonality of the emission. A comparison with air mass trajectories must allow the modelling of long distance transport

This technological program aims to get a better view of the Corbel site quality (78 54 N, 12 07 E, Svalbard close to Ny Alesunsd) for atmospheric chemistry. Nox and SO2 samplers are deployed on 16 places on a 4 km2 area around the Station (79°N, Svalbard), protected from snowscooters activity. The influence of Ny Alesund village is also studied. Programme 2004 April 2004 : poles installation and samplers deployment on the 16 stations; analysis will be made by CNR.

It is well known that the atmosphere is a conveyor of microorganisms, and that bacteria can act as ice or cloud condensation nuclei, but clouds have not been considered as a site where organisms can live and reproduce. We could show that bacteria in cloud droplets collected at high altitudes are actively growing and reproducing at temperatures at or below 0°C. Since ~60% of the earth surface is covered by clouds, cloud water should be considered as a microbial habitat.

The project aims at producing an ENVISAT-1 mission-long monitoring of the inorganic chlorine (Cly) and fluorine (Fy) loading in the Earth’s middle atmosphere, based on FTIR vertical column abundance measurements of the key related species HCl, ClONO2, HF and COF2 at 10 ground-based NDSC sites distributed worldwide. These Cly and Fy inventories will be completed with ClO and OClO measurements expected as Level-2 products from ENVISAT-1. The column abundances of the source gases CFC-12 and HCFC-22 will be used to place the stratospheric Cly and Fy evolution in perspective with the more complete sets of organic chlorinated and fluorinated compounds measured at the ground by the in situ networks NOAA-CMDL and AGAGE. The assimilation of the retrieved geophysical data bases will be performed through 3-D model calculations incorporating physical, chemical and transport characteristics of the global atmosphere.

The present project aims at the geophysical validation, from pole to pole and on the long term, of key ozone-related level-2 products (O3, NO2, BrO, OClO, and ClO) from GOMOS, MIPAS and SCIAMACHY onboard ENVISAT-1, and at a contribution to the maturation of the related level-1b-to-2 data processors. Application data processing will be used to convert level-2 data into a more suitable format for validation and scientific end-users. The respective performances of the ENVISAT data products, and their sensitivity to various relevant parameters, will be investigated from the Arctic to the Antarctic, over a variety of geophysical conditions. The impact of these performances on specific atmospheric chemistry studies will be emphasised. The pseudo-global investigations will rely on correlative studies of ENVISAT data with high-quality ground-based, in situ and balloon observations associated with the Network for the Detection of Stratospheric Change (NDSC).

The project will provide a long-term, pseudo-global validation support to the ENVISAT-1 atmospheric measurements, based on mutually consistent high-quality solar and lunar observations from FTIR spectrometers operated at primary and a number of complementary NDSC stations. The validation is limited to a number of target species, most of which are primary NRT or OL level-2 products of the mission, with focus on NOy components: O3, NO2, NO, N2O, HNO3, HNO4, H2CO, CO and CH4. Synergistic use will be made of column and profile data from MIPAS, GOMOS and SCIAMACHY. The ground network will deliver mean vertical column abundances for all target species with NDSC-type quality, and height profile information for some target gases as secondary products to the PI's home institute, where the correlative analyses with the ENVISAT-1 products will be done. Asynoptic mapping tools will support the validation efforts.

The main objectives of ESAC II are the following: (1) Extend and improve the important existing Belgian contribution in atmospheric research started in the 50s, recognized internationally. (2) Investigate the chemistry of the atmosphere, to detect and understand its evolution, mainly with experimental means. Special attention will be paid to the evolution of the ozone layer and chemical species and processes with an impact on climate changes. (3) Support the Belgian policies and decisions regarding the Amendments to: - the Montreal Protocol on Substances that deplete the Ozone Layer; - the Kyoto Protocol on Greenhouse Gases (GHG) emissions.

EARLINET will establish a quantitative comprehensive statistical database of the horizontal, vertical, and temporal distribution of aerosols on a continental scale. The goal is to provide aerosol data with unbiased sampling, for important selected processes, and air-mass history, together with comprehensive analyses of these data. The objectives will be reached by implementing a network of 21 stations distributed over most of Europe, using advanced quantitative laser remote sensing to directly measure the vertical distribution of aerosols, supported by a suite of more conventional observations. Special care will be taken to assure data quality, including intercomparisons at instrument and evaluation levels. A major part of the measurements will be performed according to a fixed schedule to provide an unbiased statistically significant data set. Additional measurements will be performed to specifically address important processes that are localised either in space or time. Back-trajectories derived from operational weather prediction models will be used to characterise the history of the observed air parcels, accounting explicitly for the vertical distribution.

SOGE is an integrated system for observation of halogenated greenhouse gases in Europe. There are two objectives: (1) To develop a new cost-effective long-term European observation system for halocarbons. The results will be in support of the Kyoto and the Montreal protocols,in assessing the compliance of European regions with the protocol requirements. In particular the observation system will be set up to: - detect trends in the concentrations of greenhouse active and ozone-destroying halocarbons; - verify reported emissions and validate emission inventories; - develop observational capacity for all halocarbons included in the Kyoto protocol (PFC, SF6) for which this is presently not yet existing; - develop a strategy for a cost-effective long-term observation system for halocarbons in Europe. (2) To predict and assess impacts of the halocarbons on the climate and on the ozone layer. This implies extensive exploitation of existing data. The impact assessment will be aimed at providing guidance for development of the Kyoto protocol and to the further development of the Montreal protocol mendments, by: - modelling impacts of halocarbons on radiative forcing and their relative importance for climate change; - modelling impacts of emissions of CFCs and HCFCs on the ozone layer.

The aim of QUILT is to optimise the exploitation of the existing European UV-visible monitoring systems by which O3 and the related free radicals NO2, BrO and OClO can be measured. These monitoring systems include ground-based, balloon and satellite observations. QUILT is providing an assessment of the chemical ozone loss over the last decade and through 2000-2003. This is achieved through analysis improvements, consolidation of existing datasets and near real time integrations with chemical transport models.

The goals of this experiment are to map out the chemical changes in the free troposphere as the atmosphere transitions from winter to spring. It is hoped to begin to understand the chemical conditions that influence the lifetime of ozone and understand more about the productivity of this region of the atmosphere with respect to the in-situ production of ozone. How the free troposphere responds to changing levels of pollution could be critical to the development of future abatement strategies.

The overall objective of COSE is to provide the Earth Observation (EO) user community with a validated, consistent and well-documented data set of mainly stratospheric constituent columns and/or profiles, by co-ordination of ground-based observations at existing stations in Europe. The data set builds on past and ongoing time series, and will be archived in a dedicated database for immediate and future exploitation, e.g., satellite validation activities, data assimilation and scientific studies. Active participation of some representative EO customers will assure that the delivered data sets come up to their requirements.

The main specific objectives of UFTIR are: (1) To revise and homogenise the analyses of available experimental data for providing consistent time series of distinct tropospheric and stratospheric abundances of the target gases using new inversion algorithms. A common strategy for retrieval and characterisation of the vertical distributions of the target gases from FTIR ground-based measurements will be established. (2) To provide quantitative trends and associated uncertainties for the target gases over about the last decade, as a function of latitude throughout Western Europe, focusing on the troposphere. (3) To integrate the data in model assessments of the evolutions of tropospheric abundances. The measured burden and changes of the tropospheric gases will be compared with 3D model simulations, in order to help developing the latter, assist in explaining potential causes for the observed changes and to assess the consistencies between the trends at the surface to the free troposphere and lowermost stratosphere, and the agreement with known evolutions of emissions. UFTIR will make the community prepared to deliver tropospheric data for validation and synergistic exploitation of new satellite experiments like ENVISAT.

A millimeter wave radiometer is started operation at the Swedish Institute of Space Physics, Kiruna, Sweden. The location of the instrument (67.8 N, 20.4 E) allows continuous observation of the evolution of ozone and ozone related trace gases in the Arctic polar stratosphere. It is designed for measurements of thermal emission lines around 204 Ghz. At this frequency observations include of ozone, chlorine monoxide, nitrous oxide, and nitric acid.

The DOAS instrument consists of grating spectrometer covering the visible and near ultraviolet spectral region. Zenith-scattered sunlight is collected by simple one-lens telescopes and fed via optical fiber bundles into the spectrometers, where atmospheric absorption spectra are obtained. The instrument runs automatically. Total column densities of the stratospheric trace species ozone, NO2, BrO, and OClO are retrieved from the spectra using the DOAS algorithm. These are species that play a major role in ozone chemistry, either by themselves in ozone destruction (BrO) or as indicators of chlorine activation/deactivation (OClO). The chemistry and dynamics of ozone destruction is investigated, e.g. with respect to the location of the polar vortex during the winter. The instrument is also useful for detection of polar stratospheric clouds using the zenith-sky colour index method.

FT-IR spectrometers are capable to quantifiy the total column amounts of many important trace gases in the troposphere and stratosphere. At present the following species are retrieved from the Kiruna data: O3 (ozone), ClONO2, HNO3, HCl, CFC-11, CFC-12, CFC-22, NO2, N2O, NO, HF, C2H2, C2H4, C2H6, CH4, CO, COF2, H2O, HCN, HO2NO2, NH3, N2, and OCS Selected research topics and activities: chemical ozone depletion by observation of key species (O3, ClONO2, HNO3, HCl, ..) details of the ozone formation process by isotopic studies in ozone profile retrieval to detect dynamical changes transport studies of chemical tracers and tropospheric pollutants satellite validation

FT-IR spectrometers are capable to quantifiy the total column amounts of many important trace gases in the troposphere and stratosphere. At present the following species are retrieved from the Kiruna data: O3 (ozone), ClONO2, HNO3, HCl, CFC-11, CFC-12, CFC-22, NO2, N2O, NO, HF, C2H2, C2H4, C2H6, CH4, CO, COF2, H2O, HCN, HO2NO2, NH3, N2, and OCS Selected research topics and activities: chemical ozone depletion by observation of key species (O3, ClONO2, HNO3, HCl, ..) details of the ozone formation process by isotopic studies in ozone profile retrieval to detect dynamical changes transport studies of chemical tracers and tropospheric pollutants satellite validation

Objective: to collect climatology information on the seasonal and year-to-tear variability of stratospheric CFCs, water vapour and atmospheric electrical parameters.